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According to the episode guides, while in Barcelona they stayed at the AC Miramar on MontjuÏc and dined at the now closed Inopia, at Bar Pinotxo in the Boquería and La Clara on Gran Vía les Corts Catalanes 445.
You can see where they dined outside of Barcelona by clicking on the Spain map here-
Can Jubany, Carme Ruscalleda, as mentioned, and Rafa's in Roses in Catalunya.
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